Publications since joining NUS

90

Du, Y.; Yao, B.; Xu, L.; Lu, S.; Xu, C.; Han, P.; Dai, S.; Wang, S.; Xi, S.; Neo, B. S.; Yan, N.*; He, Q*. Single-Atom Catalysts Enabled Catalytic Ammonia Combustion at 1,100°C. Joule 2025, No. 102030.

89

Zhao, B.; Zou, J.; Yao, B.; Wade, A.; Liu, L.*; Dong, J.; He, Q.* Fabricating Hydrogen-Rich Microenvironment through Dual-Site Catalysts for Boosting Glycerol Selective Hydrogenolysis. Appl. Catal. B 2025, 377 (125464), 125464.

88

Indriadi, K. S.; Du, Y.; He, Q.*; Yan, N.* Critical Downstream Catalytic Processes for an NH3 Economy. Appl. Energy 2025, 393 (126099), 126099.

87

Yao, B.; Xu, C.; Tang, Y.; Du, Y.; Tan, S.; Dai, S.; Luo, G.; He, Q.* Harnessing Zn-Volatility for Compositional Tuning in PtZn Nanoalloy Catalysts. Nano Today 2025, 63 (102746), 102746.

86

Chen, J.; Liu, C.; Xi, S.; Tan, S.; He, Q.; Liang, L.; Liu, X. Optical Nonlinearities in Excess of 500 through Sublattice Reconstruction. Nature 2025, 1–6.

85

Tang, X.; Ge, S.; Lv, Y.; Sun, G.; Wang, Z.; Xie, J.; Peng, M.; Xu, Y.; Zhang, J.; Yao, B.; He, Q.; Guo, Y.; Zhan, W.; Wang, L.; Zhou, L.; Xu, B.; Dai, S.; Guo, Y.; Ma, D. Blocking the Operando Formation of Single-Atom Spectators by Interfacial Engineering. Angew. Chem. Int. Ed Engl. 2025, 64 (23), e202505507.

84

Gao, Q.; Yao, B.; Liu, Y.; Shi, L.; Yan, Z.; Xu, L.; He, Q.*; Zhu, H.* Strain Relaxation Enhances Ammonia Electrosynthesis from Nitrate on Cu/CuAu Core/Shell Nanocrystals with Ordered Intermetallic Layers. Chem Catal. 2025, 5 (6), 101328.

83

Yang, J.; Falling, L. J.; Yan, S.; Zhang, B.; Verma, P.; Daemen, L.; Cheng, Y.; Zhao, X.; Zhang, S.; Chen, J.-L.; Yao, B.; Tan, S.; Chae, S.; He, Q.; Nemsak, S.; Wu, Z.; Prendergast, D.; Guo, Y.; Liu, J.; Salmeron, M.; Su, J. Formation of Hydrided Pt-Ce-H Sites in Efficient, Selective Oxidation Catalysts. Science 2025, 388 (6746), 514–519.

82

Shi, J.; Wang, G.; Tian, D.; Hai, X.; Meng, R.; Xu, Y.; Teng, Y.; Ma, L.; Xi, S.; Yang, Y.; Zhou, X.; Fu, X.; Li, H.; Cai, Q.; He, P.; Lin, H.; Chen, J.; Li, J.; Li, J.; He, Q.; Yang, Q.-H.; Li, J.; Wu, D.; Wang, Y.-G.; Wu, J.; Lu, J. Defying the Oxidative-Addition Prerequisite in Cross-Coupling through Artful Single-Atom Catalysts. Nat. Commun. 2025, 16 (1), 3223.

81

Pei, X.; Su, M.; Waldron, C.; Walker, M.; Decarolis, D.; He, Q.; Archer, S.; Smith, M. B.; Dann, S. E.; Kondrat, S. A. Enhanced Stability and Activity in the Upgrading Ethanol to N-Butanol Using a Ruthenium Polyphenylene Catalyst. Appl. Catal. A Gen. 2025, 694 (120139), 120139.

80

He, J.; Liang, Y.; Zhao, B.; Liu, L.*; He, Q.*; Wang, D.; Dong, J.* Isomorphous Substitution in CaAl-Hydrotalcite to Construct High Density Single-Atom Catalysts for Selective N-Heteroarene Hydrogenation. Cuihua Xuebao/Chin. J. Catalysis 2025, 70, 353–362.

79

Tang, Y.; Hou, M.; He, Q.*; Luo, G*. Designing Bimetallic Nanoparticle Catalysts via Tailored Surface Segregation. Nano Lett. 2025, 25 (6), 2459–2465.

78

Mu, C.; Liu, Z.; Yao, Q.; He, Q.*; Xie, J.* Engineering Metal Nanoclusters at the Atomic Level for Effective Electrocatalysis. SmartMat 2025, 6 (1). https://doi.org/10.1002/smm2.1317.

77

Jin, H.; Chen, X.; Da, Y.; Fan, L.; Jiang, R.; Xiao, Y.; Yao, B.; He, Q.; Yu, Y.; Chen, W. Identifying the Bifunctional Mechanism in Alkaline Water Electrolysis by Lewis Pairs at the Single-Atom Scale. J. Am. Chem. Soc. 2025, 147 (4), 3874–3884.

76

Wu, Y.; Nguyen, P. T. T.; Wong, S. S.; Feng, M.; Han, P.; Yao, B.; He, Q.; Sum, T. C.; Zhang, T.; Yan, N. Photocatalytic Upcycling of Polylactic Acid to Alanine by Sulfur Vacancy-Rich Cadmium Sulfide. Nat. Commun. 2025, 16 (1), 846.

75

Liu, S.; Shi, C.; Xu, C.; Zhang, H.; Li, W.; Briega-Martos, V.; He, Q.; Han, Y.; Yang, Y. Epitaxial Growth of Atomic-Layer Cu on Pd Nanocatalysts for Electrochemical CO₂ Reduction. Chem. Mater. 2024, 37 (1), 290–296.

74

Deng, C.; Liu, R.; Wu, P.; Wang, T.; Xi, S.; Tao, D.; He, Q.; Chao, Y.; Zhu, W.; Dai, S. Thermally Stable High-Entropy Layered Double Hydroxides for Advanced Catalysis. Small 2024, 20 (51), e2406685.

73

Mu, C.; Wang, B.; Yao, Q.; He, Q.*; Xie, J. Composition-Dependent Catalytic Performance of AuxAg25-x Alloy Nanoclusters for Oxygen Reduction Reaction. Nano Res. 2024, 17 (11), 9490–9497.

72

Song, W.; Wang, C.; Liu, Y.; Chong, K. C.; Zhang, X.; Wang, T.; Zhang, Y.; Li, B.; Tian, J.; Zhang, X.; Wang, X.; Yao, B.; Wang, X.; Xiao, Y.; Yao, Y.; Mao, X.; He, Q.; Lin, Z.; Zou, Z.; Liu, B. Unlocking Copper-Free Interfacial Asymmetric C-C Coupling for Ethylene Photosynthesis from CO2 and H2O. J. Am. Chem. Soc. 2024, 146 (42), 29028–29039.

71

Yang, Y.; Wu, L.; Yao, B.; Zhang, L.; Jung, M.; He, Q.; Yan, N.; Liu, C.-J. Gallium Cluster-Promoted in₂O₃ Catalyst for CO₂ Hydrogenation to Methanol. ACS Catal. 2024, 14 (18), 13958–13972.

70

Yang, H.; Guo, N.; Xi, S.; Wu, Y.; Yao, B.; He, Q.; Zhang, C.; Wang, L. Potential-Driven Structural Distortion in Cobalt Phthalocyanine for Electrocatalytic CO2/CO Reduction towards Methanol. Nat. Commun. 2024, 15 (1), 7703.

69

Yuan, W.; Peng, C.; He, Q.* A Large Language Model-Powered Literature Review for High-Angle Annular Dark Field Imaging. Chin. Physics B 2024, 33 (9), 098703.

68

Zeng, S.; Tang, C. S.; Luo, Z.; Chow, L. E.; Lim, Z. S.; Prakash, S.; Yang, P.; Diao, C.; Yu, X.; Xing, Z.; Ji, R.; Yin, X.; Li, C.; Wang, X. R.; He, Q.; Breese, M. B. H.; Ariando, A.; Liu, H. Origin of a Topotactic Reduction Effect for Superconductivity in Infinite-Layer Nickelates. Phys. Rev. Lett. 2024, 133 (6), 066503.

67

Fan, Q.; Tan, M.; Yao, B.; Saqline, S.; Tao, L.; He, Q.; Liu, W. Synthesis of Uniform Fe2O3@Y2O3 Yolk−shell Nanoreactors as Chemical Looping Oxygen Carriers. Appl. Catal. B 2024, 350 (123935), 123935.

66

Lan, D.*; Yao, B.; Swamynadhan, M. J.; Li, N.; Cao, J.; Shi, S.; Yu, X.; Yang, P.; Wu, X.; Liu, C.; Chen, P.; Chen, J.; Ghosh, S.; He, Q.* Interfacial Electronic and Magnetic Reconstructions in Manganite/Titanate Superlattices. Adv. Mater. Interfaces 2024, 11 (19). https://doi.org/10.1002/admi.202300903.

65

Xu, C.; Yao, B.; He, Q.* Complex-Assisted PtZn Alloy Formation for Propane Dehydrogenation. ARKIVOC 2024, 2024 (3). https://doi.org/10.24820/ark.5550190.p012.190.

64

Liu, S.; Li, Y.; Wang, D.; Xi, S.; Xu, H.; Wang, Y.; Li, X.; Zang, W.; Liu, W.; Su, M.; Yan, K.; Nielander, A. C.; Wong, A. B.; Lu, J.; Jaramillo, T. F.; Wang, L.*; Canepa, P.*; He, Q.* Alkali Cation-Induced Cathodic Corrosion in Cu Electrocatalysts. Nat. Commun. 2024, 15 (1), 5080.

63

Wang, D.; Jung, H. D.; Liu, S.; Chen, J.; Yang, H.; He, Q.*; Xi, S.*; Back, S.*; Wang, L.* Revealing the Structural Evolution of CuAg Composites during Electrochemical Carbon Monoxide Reduction. Nat. Commun. 2024, 15 (1), 4692.

62

Wang, S.; An, H.; Hülsey, M. J.; Sun, G.; He, Q.*; Yan, N.* Sulfite-Enhanced Aerobic Methane Oxidation to Methanol over Reduced Phosphomolybdate. ACS Catal. 2024, 14 (6), 4352–4361.

61

Li, J.; Chen, Y.; Yao, B.; Yang, W.; Cui, X.; Liu, H.; Dai, S.; Xi, S.; Sun, Z.; Chen, W.; Qin, Y.; Wang, J.; He, Q.*; Ling, C.; Wang, D.; Zhang, Z. Cascade Dual Sites Modulate Local CO Coverage and Hydrogen-Binding Strength to Boost CO2 Electroreduction to Ethylene. J. Am. Chem. Soc. 2024, 146 (8), 5693–5701.

60

Cao, J.; Qi, G.; Yao, B.; He, Q.; Lewis, R. J.; Li, X.; Deng, F.; Xu, J.; Hutchings, G. J. Partially Bonded Aluminum Site on the External Surface of Post-Treated Au/ZSM-5 Enhances Methane Oxidation to Oxygenates. ACS Catal. 2024, 14 (3), 1797–1807.

59

Xu, C.; Tan, S.; Tang, Y.; Xi, S.; Yao, B.; Wade, A.; Zhao, B.; Lu, S.; Du, Y.; Tian, M.; He, C.; Ma, L.; Fu, X.; Shi, J.; Lu, J.; Howe, A. G. R.; Dai, S.; Luo, G.; He, Q.* Compositional Variations in Highly Active PtSn/Al2O3 Catalysts Derived from Molecular Complexes. Appl. Catal. B 2024, 341 (123285), 123285.

58

Nguyen, P. T. T.; Gözaydın, G.; Ma, J.; Yao, B.; He, Q.; Yan, N. Direct Amination of Poly(p-Phenylene Oxide) to Substituted Anilines over Bimetallic Pd–Ru Catalysts. Green Chem. 2024, 26 (7), 3949–3957.

57

Zhou, L.; Liang, L.; Chen, J.; Zhou, X.; Liu, L.; Xi, S.; Loh, K. P.; Han, Y.; He, Q.*; Liu, X.* Promoted Growth and Multiband Emission in Heterostructured Perovskites through Cs+ -Sublattice Interaction. Adv. Sci. (Weinh.) 2024, 11 (3), e2306398.

56

Wang, L.; Zhou, X.; Su, M.; Zhang, Y.; Li, R.; Zhang, R.; Wu, X.; Wu, Z.; Wong, W. P. D.; Xu, Q.-H.; He, Q.; Loh, K. P. In-Plane Ferrielectric Order in van Der Waals β’-In2Se3. ACS Nano 2023, 18 (1), 809–818.

55

Zhao, B.; Zou, J.; Chen, C.; He, Q.; Tang, Q.; Liu, L.; Dong, J. Single Tungsten Atom-Modified Pt/Al2O3 to Boost Glycerol Hydrogenolysis to 1,3-Propanediol. Chem. Eng. J. 2023, 478 (147396), 147396.

54

Waqar, M.; Chai, J.; Wong, L. M.; Lim, P. C.; Chen, S.; Liew, W. H.; Wang, S.; Chen, J.; He, Q.; Yao, K.; Wang, J. Large Electromechanical Response in a Polycrystalline Alkali-Deficient (K,Na)NbO3 Thin Film on Silicon. Nano Lett. 2023, 23 (23), 11026–11033.

53

Miao, C.; Liu, M.; Tan, S.; Zhang, G.; Chu, S.; Song, S.; Zhang, Q.; Yu, J.; Jiang, G.; Song, W.; He, Q.*; Luo, W.; Wu, Z. Pt–Sn Nanoalloys on Sn-Beta Zeolite for Efficient Propane Dehydrogenation. Microporous Mesoporous Mater. 2023, 361 (112736), 112736.

52

Gao, Q.; Yan, Z.; Zhang, W.; Pillai, H. S.; Yao, B.; Zang, W.; Liu, Y.; Han, X.; Min, B.; Zhou, H.; Ma, L.; Anaclet, B.; Zhang, S.; Xin, H.*; He, Q.*; Zhu, H.* Atomic Layers of B2 CuPd on Cu Nanocubes as Catalysts for Selective Hydrogenation. J. Am. Chem. Soc. 2023, 145 (36), 19961–19968.

51

Parker, L. A.; Richards, N.; Bailey, L.; Carter, J. H.; Nowicka, E.; Pattisson, S.; Dummer, N. F.; He, Q.; Lu, L.; Kiely, C. J.; Golunski, S. E.; Roldan, A.; Hutchings, G. J. Investigating Periodic Table Interpolation for the Rational Design of Nanoalloy Catalysts for Green Hydrogen Production from Ammonia Decomposition. Catal. Letters 2023, 154 (5), 1958–1969.

50

Wang, S.; Fung, V.; Hülsey, M. J.; Liang, X.; Yu, Z.; Chang, J.; Folli, A.; Lewis, R. J.; Hutchings, G. J.; He, Q.*; Yan, N.* H2-Reduced Phosphomolybdate Promotes Room-Temperature Aerobic Oxidation of Methane to Methanol. Nat. Catal. 2023, 6 (10), 895–905.

49

Chen, J.; Liang, L.; Tan, S.; Xi, S.; Lin, C.-H.; Wu, T.; He, Q.; Liu, X. Volumetric Nanocrystal Lattice Reconstruction through Dynamic Metal Complex Docking. Nano Lett. 2023, 23 (15), 7221–7227.

48

Liang, Z.; Zhou, X.; Zhang, L.; Yu, X.-L.; Lv, Y.; Song, X.; Zhou, Y.; Wang, H.; Wang, S.; Wang, T.; Shum, P. P.; He, Q.; Liu, Y.; Zhu, C.; Wang, L.; Chen, X. Strong Bulk Photovoltaic Effect in Engineered Edge-Embedded van Der Waals Structures. Nat. Commun. 2023, 14 (1), 4230.

47

Indriadi, K. S.; Han, P.; Ding, S.; Yao, B.; Furukawa, S.; He, Q.*; Yan, N.* Highly Dispersed Pt Boosts Active Fe N Formation in Ammonia Decomposition. Cuihua Xuebao/Chin. J. Catalysis 2023, 50, 297–305.

46

Sun, T.; Tang, Z.; Zang, W.; Li, Z.; Li, J.; Li, Z.; Cao, L.; Dominic Rodriguez, J. S.; Mariano, C. O. M.; Xu, H.; Lyu, P.; Hai, X.; Lin, H.; Sheng, X.; Shi, J.; Zheng, Y.; Lu, Y.-R.; He, Q.; Chen, J.; Novoselov, K. S.; Chuang, C.-H.; Xi, S.; Luo, X.; Lu, J. Ferromagnetic Single-Atom Spin Catalyst for Boosting Water Splitting. Nat. Nanotechnol. 2023, 18 (7), 763–771.

45

Das, S.; Anjum, U.; Lim, K. H.; He, Q.; Hoffman, A. S.; Bare, S. R.; Kozlov, S. M.; Gates, B. C.; Kawi, S. Genesis of Active Pt/CeO2 Catalyst for Dry Reforming of Methane by Reduction and Aggregation of Isolated Platinum Atoms into Clusters. Small 2023, 19 (26), e2207272.

44

Cao, J.; Lewis, R. J.; Qi, G.; Bethell, D.; Howard, M. J.; Harrison, B.; Yao, B.; He, Q.; Morgan, D. J.; Ni, F.; Sharma, P.; Kiely, C. J.; Li, X.; Deng, F.; Xu, J.; Hutchings, G. J. Methane Conversion to Methanol Using Au/ZSM-5 Is Promoted by Carbon. ACS Catal. 2023, 13 (11), 7199–7209.

43

Ning, S.; Xu, W.; Loh, L.; Lu, Z.; Bosman, M.; Zhang, F.; He, Q.* An Integrated Constrained Gradient Descent (iCGD) Protocol to Correct Scan-Positional Errors for Electron Ptychography with High Accuracy and Precision. Ultramicroscopy 2023, 248, 113716.

42

Dummer, N. F.; Willock, D. J.; He, Q.; Howard, M. J.; Lewis, R. J.; Qi, G.; Taylor, S. H.; Xu, J.; Bethell, D.; Kiely, C. J.; Hutchings, G. J. Methane Oxidation to Methanol. Chem. Rev. 2023, 123 (9), 6359–6411.

41

Gao, Q.; Yao, B.; Pillai, H. S.; Zang, W.; Han, X.; Liu, Y.; Yu, S.-W.; Yan, Z.; Min, B.; Zhang, S.; Zhou, H.; Ma, L.; Xin, H.*; He, Q.*; Zhu, H.* Synthesis of Core/Shell Nanocrystals with Ordered Intermetallic Single-Atom Alloy Layers for Nitrate Electroreduction to Ammonia. Nat. Synth. 2023, 2 (7), 624–634.

40

Zhao, L.; Akdim, O.; Huang, X.; Wang, K.; Douthwaite, M.; Pattisson, S.; Lewis, R. J.; Lin, R.; Yao, B.; Morgan, D. J.; Shaw, G.; He, Q.; Bethell, D.; McIntosh, S.; Kiely, C. J.; Hutchings, G. J. Insights into the Effect of Metal Ratio on Cooperative Redox Enhancement Effects over Au- and Pd-Mediated Alcohol Oxidation. ACS Catal. 2023, 13 (5), 2892–2903.

39

Waqar, M.; He, Q.; Chai, J.; Lim, P. C.; Yao, K.; Wang, J. Diverse Defects in Alkali Niobate Thin Films: Understanding at Atomic Scales and Their Implications on Properties. Small 2023, 19 (4), e2205137.

38

Zhong, H.; Wang, X.; Sun, G.; Tang, Y.; Tan, S.; He, Q.; Zhang, J.; Xiong, T.; Diao, C.; Yu, Z.; Xi, S.; Lee, W. S. V.; Xue, J. Optimization of Oxygen Evolution Activity by Tuning Band Broadening in Nickel Oxyhydroxide. Energy Environ. Sci. 2023, 16 (2), 641–652.

37

Xu, R.; Kang, L.; Papanikolaou, K. G.; Wang, B.; Marlow, S.; He, Q.; Zhang, P.; Wang, J.; Brett, D. J. L.; Stamatakis, M.; Wang, F. R. Improving the ORR Performance by Enhancing the Pt Oxidation Resistance. J. Catal. 2022, 416, 311–321.

36

Waqar, M.; Yang, P.; He, Q.; Yao, K.; Wang, J. Negative Capacitance Phenomenon and Origin in Alkali Niobate Film with Self‐assembled Lattice Faults. Adv. Electron. Mater. 2022, 8 (11), 2200633.

35

Yan, Z.; Yao, B.; Hall, C.; Gao, Q.; Zang, W.; Zhou, H.*; He, Q.*; Zhu, H.* Metal-Metal Oxide Catalytic Interface Formation and Structural Evolution: A Discovery of Strong Metal-Support Bonding, Ordered Intermetallics, and Single Atoms. Nano Lett. 2022, 22 (20), 8122–8129.

34

Li, Z.; Jiang, J.; Liu, X.; Zhu, Z.; Wang, J.; He, Q.; Kong, Q.; Niu, X.; Chen, J. S.; Wang, J.; Wu, R. Coupling Atomically Dispersed Fe-N5 Sites with Defective N-Doped Carbon Boosts CO2 Electroreduction. Small 2022, 18 (38), e2203495.

33

Waqar, M.; Wu, H.; Ong, K. P.; Liu, H.; Li, C.; Yang, P.; Zang, W.; Liew, W. H.; Diao, C.; Xi, S.; Singh, D. J.; He, Q.; Yao, K.; Pennycook, S. J.; Wang, J. Origin of Giant Electric-Field-Induced Strain in Faulted Alkali Niobate Films. Nat. Commun. 2022, 13 (1), 3922.

32

Yan, Y.; Wong, R. J.; Ma, Z.; Donat, F.; Xi, S.; Saqline, S.; Fan, Q.; Du, Y.; Borgna, A.; He, Q.; Müller, C. R.; Chen, W.; Lapkin, A. A.; Liu, W. CO2 Hydrogenation to Methanol on Tungsten-Doped Cu/CeO2 Catalysts. Appl. Catal. B 2022, 306 (121098), 121098.

31

Li, X.; Guo, N.; Chen, Z.; Zhou, X.; Zhao, X.; Du, Y.; Ma, L.; Fang, Y.; Xu, H.; Yang, H.; Yu, W.; Lu, S.; Tian, M.; He, Q.; Loh, K. P.; Xi, S.; Zhang, C.; Lu, J. Atomically Precise Single Metal Oxide Cluster Catalyst with Oxygen‐controlled Activity. Adv. Funct. Mater. 2022, 32 (25), 2200933.

30

Yang, H.; Zhang, T.; Chi, X.; Yu, X.; Chen, J.; Chen, J.; Li, C.; Tan, S.; He, Q.; Wang, X.; Wang, L. Promoting Oxygen Reduction via Coordination Environment Modulation through Secondary Metal-Atom Incorporation. J. Mater. Chem. A Mater. Energy Sustain. 2022, 10 (37), 19626–19634.

29

Han, X.; Mou, T.; Liu, S.; Ji, M.; Gao, Q.; He, Q.; Xin, H.; Zhu, H. Heterostructured Bi-Cu2S Nanocrystals for Efficient CO2 Electroreduction to Formate. Nanoscale Horiz 2022, 7 (5), 508–514.

28

Lee, K.; Anjum, U.; Araújo, T. P.; Mondelli, C.; He, Q.; Furukawa, S.; Pérez-Ramírez, J.; Kozlov, S. M.; Yan, N. Atomic Pd-Promoted ZnZrO Solid Solution Catalyst for CO2 Hydrogenation to Methanol. Appl. Catal. B 2022, 304 (120994), 120994.

27

Gao, Q.; Pillai, H. S.; Huang, Y.; Liu, S.; Mu, Q.; Han, X.; Yan, Z.; Zhou, H.; He, Q.*; Xin, H.*; Zhu, H.* Breaking Adsorption-Energy Scaling Limitations of Electrocatalytic Nitrate Reduction on Intermetallic CuPd Nanocubes by Machine-Learned Insights. Nat. Commun. 2022, 13 (1), 2338.

26

Li, D.; Zhu, B.; Backes, D.; Veiga, L. S. I.; Lee, T.-L.; Wang, H.; He, Q.; Roy, P.; Zhang, J.; Shi, J.; Chen, A.; van Aken, P. A.; Jia, Q.; Dhesi, S. S.; Scanlon, D. O.; Zhang, K. H. L.; Li, W. Manipulating the Metal-to-Insulator Transition and Magnetic Properties in Manganite Thin Films via Epitaxial Strain. Phys. Rev. B. 2022, 105 (16). https://doi.org/10.1103/physrevb.105.165426.

25

Paris, C. B.; Howe, A. G.; Lewis, R. J.; Hewes, D.; Morgan, D. J.; He, Q.; Edwards, J. K. Impact of the Experimental Parameters on Catalytic Activity When Preparing Polymer Protected Bimetallic Nanoparticle Catalysts on Activated Carbon. ACS Catal. 2022, 12 (8), 4440–4454.

24

Dan, J.; Zhao, X.; Ning, S.; Lu, J.; Loh, K. P.; He, Q.; Loh, N. D.; Pennycook, S. J. Learning Motifs and Their Hierarchies in Atomic Resolution Microscopy. Sci. Adv. 2022, 8 (15), eabk1005.

23

Huang, X.; Akdim, O.; Douthwaite, M.; Wang, K.; Zhao, L.; Lewis, R. J.; Pattisson, S.; Daniel, I. T.; Miedziak, P. J.; Shaw, G.; Morgan, D. J.; Althahban, S. M.; Davies, T. E.; He, Q.; Wang, F.; Fu, J.; Bethell, D.; McIntosh, S.; Kiely, C. J.; Hutchings, G. J. Au-Pd Separation Enhances Bimetallic Catalysis of Alcohol Oxidation. Nature 2022, 603 (7900), 271–275.

22

Ning, S.; Xu, W.; Ma, Y.; Loh, L.; Pennycook, T. J.; Zhou, W.; Zhang, F.; Bosman, M.; Pennycook, S. J.; He, Q.*; Loh, N. D.* Accurate and Robust Calibration of the Uniform Affine Transformation between Scan-Camera Coordinates for Atom-Resolved in-Focus 4D-STEM Datasets. Microsc. Microanal. 2022, 28 (3), 1–11.

21

Qi, G.; Davies, T. E.; Nasrallah, A.; Sainna, M. A.; Howe, A. G. R.; Lewis, R. J.; Quesne, M.; Catlow, C. R. A.; Willock, D. J.; He, Q.; Bethell, D.; Howard, M. J.; Murrer, B. A.; Harrison, B.; Kiely, C. J.; Zhao, X.; Deng, F.; Xu, J.; Hutchings, G. J. Au-ZSM-5 Catalyses the Selective Oxidation of CH4 to CH3OH and CH3COOH Using O2. Nat. Catal. 2022, 5 (1), 45–54.

20

Ding, S.; Hülsey, M. J.; An, H.; He, Q.; Asakura, H.; Gao, M.; Hasegawa, J.-Y.; Tanaka, T.; Yan, N. Ionic Liquid-Stabilized Single-Atom Rh Catalyst against Leaching. CCS Chem 2021, 3 (10), 1814–1822.

19

Richards, T.; Harrhy, J. H.; Lewis, R. J.; Howe, A. G. R.; Suldecki, G. M.; Folli, A.; Morgan, D. J.; Davies, T. E.; Loveridge, E. J.; Crole, D. A.; Edwards, J. K.; Gaskin, P.; Kiely, C. J.; He, Q.; Murphy, D. M.; Maillard, J.-Y.; Freakley, S. J.; Hutchings, G. J. A Residue-Free Approach to Water Disinfection Using Catalytic in Situ Generation of Reactive Oxygen Species. Nat. Catal. 2021, 4 (7), 575–585.

18

Zhao, B.; Liang, Y.; Liu, L.*; He, Q.*; Dong, J.-X. Facilitating Pt−WO x Species Interaction for Efficient Glycerol Hydrogenolysis to 1,3‐propanediol. ChemCatChem 2021, 13 (cctc.202100773), 3695–3705.

17

Kang, L.; Wang, B.; Güntner, A. T.; Xu, S.; Wan, X.; Liu, Y.; Marlow, S.; Ren, Y.; Gianolio, D.; Tang, C. C.; Murzin, V.; Asakura, H.; He, Q.; Guan, S.; Velasco-Vélez, J. J.; Pratsinis, S. E.; Guo, Y.; Wang, F. R. The Electrophilicity of Surface Carbon Species in the Redox Reactions of CuO-CeO2 Catalysts. Angew. Chem. Int. Ed Engl. 2021, 60 (26), 14420–14428.

16

Guadix-Montero, S.; Santos Hernandez, A.; Lei, N.; Morgan, D. J.; He, Q.; Wang, A.; Zhang, T.; Roldan, A.; Sankar, M. Controlling the Selectivity of Supported Ru Nanoparticles during Glycerol Hydrogenolysis: C−O vs C−C Cleavage. ChemCatChem 2021, 13 (6), 1595–1606.

15

Fu, G.; Li, W.; Zhang, J.-Y.; Li, M.; Li, C.; Li, N.; He, Q.; Xi, S.; Qi, D.; MacManus-Driscoll, J. L.; Cheng, J.; Zhang, K. H. Facilitating the Deprotonation of OH to O through Fe⁴⁺ -Induced States in Perovskite LaNiO3 Enables a Fast Oxygen Evolution Reaction. Small 2021, 17 (12), e2006930.

14

Ding, S.; Chen, H.-A.; Mekasuwandumrong, O.; Hülsey, M. J.; Fu, X.; He, Q.; Panpranot, J.; Yang, C.-M.; Yan, N. High-Temperature Flame Spray Pyrolysis Induced Stabilization of Pt Single-Atom Catalysts. Appl. Catal. B 2021, 281 (119471), 119471.

13

Kang, L.; Wang, B.; Thetford, A.; Wu, K.; Danaie, M.; He, Q.; Gibson, E. K.; Sun, L.-D.; Asakura, H.; Catlow, C. R. A.; Wang, F. R. Design, Identification, and Evolution of a Surface Ruthenium(II/III) Single Site for CO Activation. Angew. Chem. Int. Ed Engl. 2021, 60 (3), 1212–1219.

12

Li, Q.; Wang, B.; He, Q.; Yu, P.; Chen, L.-Q.; Kalinin, S. V.; Li, J.-F. Ferroelastic Nanodomain-Mediated Mechanical Switching of Ferroelectricity in Thick Epitaxial Films. Nano Lett. 2021, 21 (1), 445–452.

11

Yu, T.; Li, Z.; Jones, W.; Liu, Y.; He, Q.; Song, W.; Du, P.; Yang, B.; An, H.; Farmer, D. M.; Qiu, C.; Wang, A.; Weckhuysen, B. M.; Beale, A. M.; Luo, W. Identifying Key Mononuclear Fe Species for Low-Temperature Methane Oxidation. Chem. Sci. 2021, 12 (9), 3152–3160.

10

Underhill, R.; Douthwaite, M.; Lewis, R. J.; Miedziak, P. J.; Armstrong, R. D.; Morgan, D. J.; Freakley, S. J.; Davies, T.; Folli, A.; Murphy, D. M.; He, Q.; Akdim, O.; Edwards, J. K.; Hutchings, G. J. Ambient Base-Free Glycerol Oxidation over Bimetallic PdFe/SiO2 by in Situ Generated Active Oxygen Species. Res. Chem. Intermed. 2021, 47 (1), 303–324.

9

Zhao, B.; Liang, Y.; Liu, L.*; He, Q.*; Dong, J. Discovering Positively Charged Pt for Enhanced Hydrogenolysis of Glycerol to 1,3-Propanediol. Green Chem. 2020, 22 (23), 8254–8259.

8

Sun, Q.; Chen, B. W. J.; Wang, N.; He, Q.; Chang, A.; Yang, C.-M.; Asakura, H.; Tanaka, T.; Hülsey, M. J.; Wang, C.-H.; Yu, J.; Yan, N. Zeolite-Encaged Pd-Mn Nanocatalysts for CO2 Hydrogenation and Formic Acid Dehydrogenation. Angew. Chem. Int. Ed Engl. 2020, 59 (45), 20183–20191.

7

Gao, Q.; Mou, T.; Liu, S.; Johnson, G.; Han, X.; Yan, Z.; Ji, M.; He, Q.; Zhang, S.; Xin, H.; Zhu, H. Monodisperse PdSn/SnOx Core/Shell Nanoparticles with Superior Electrocatalytic Ethanol Oxidation Performance. J. Mater. Chem. A Mater. Energy Sustain. 2020, 8 (40), 20931–20938.

6

Xu, H.; Xi, S.; Li, J.; Liu, S.; Lyu, P.; Yu, W.; Sun, T.; Qi, D.-C.; He, Q.; Xiao, H.; Lin, M.; Wu, J.; Zhang, J.; Lu, J. Chemical Design and Synthesis of Superior Single-Atom Electrocatalysts via in Situ Polymerization. J. Mater. Chem. A Mater. Energy Sustain. 2020, 8 (34), 17683–17690.

5

Liu, S.; Gow, I.; Davies, T.; Barnes, A.; Sankar, M.; Gong, X.; Howe, A. G. R.; Dixon, M.; Hutchings, G. J.; Kiely, C. J.; He, Q.* Probing Composition Distributions in Nanoalloy Catalysts with Correlative Electron Microscopy. J. Mater. Chem. A Mater. Energy Sustain. 2020, 8 (31), 15725–15733.

4

Kang, L.; Wang, B.; Bing, Q.; Zalibera, M.; Büchel, R.; Xu, R.; Wang, Q.; Liu, Y.; Gianolio, D.; Tang, C. C.; Gibson, E. K.; Danaie, M.; Allen, C.; Wu, K.; Marlow, S.; Sun, L.-D.; He, Q.; Guan, S.; Savitsky, A.; Velasco-Vélez, J. J.; Callison, J.; Kay, C. W. M.; Pratsinis, S. E.; Lubitz, W.; Liu, J.-Y.; Wang, F. R. Adsorption and Activation of Molecular Oxygen over Atomic Copper(I/II) Site on Ceria. Nat. Commun. 2020, 11 (1), 4008.

3

Jarvis, J. S.; Harrhy, J. H.; Wang, A.; Bere, T.; Morgan, D. J.; Carter, J. H.; Howe, A. G. R.; He, Q.; Hutchings, G. J.; Song, H. Inhibiting the Dealkylation of Basic Arenes during n-Alkane Direct Aromatization Reactions and Understanding the C₆ Ring Closure Mechanism. ACS Catal. 2020, 10 (15), 8428–8443.

2

Sankar, M.; He, Q.; Engel, R. V.; Sainna, M. A.; Logsdail, A. J.; Roldan, A.; Willock, D. J.; Agarwal, N.; Kiely, C. J.; Hutchings, G. J. Role of the Support in Gold-Containing Nanoparticles as Heterogeneous Catalysts. Chem. Rev. 2020, 120 (8), 3890–3938.

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